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Cruella de Vil
There have been many incarnations of Cruella de Vil, but each and every one had her kidnapping Dalmatian puppies for their fur. That's right: puppy fur. Naturally, this villain can't succeed, because in Disney movies puppies always win, but as an animal lover who was actually scarred the first time I saw this movie as a kid, in my mind, she's one of the greatest female villains of all time.